Unveiling the Root Cause of the Efficiency-Lifetime Trade-Off in Blue Fluorescent Organic Light-Emitting Diodes

Sunwoo Kang, Jun Yeob Lee, Taekyung Kim

Research output: Contribution to journalArticlepeer-review

20 Scopus citations

Abstract

Abstract: The origin of efficiency-lifetime trade-off in triplet–triplet fusion (TTF) type blue fluorescent organic light-emitting diodes (OLEDs) was investigated and the device structure to resolve the issue was developed. The efficiency and lifetime were simultaneously improved in the blue OLEDs by developing a multilayer hole transport stack which can adjust carrier densities and recombination zone in the emitting layer (EML). It was found that electron leakage from EML and high spatial density of excitons in the vicinity of the electron blocking layer for high TTF rates by narrow recombination zone are the detrimental factors for efficiency-lifetime trade-off. A multilayer hole transport stack employing a deep highest occupied molecular orbital hole transport layer and an electron blocking layer combined with an appropriate hole blocking layer simultaneously improved the power efficiency by 16% at 500 cd/m2 and lifetime by almost 100% (from 73 h up to 145 h). In addition, the low efficiency in the low luminance region was also completely controlled, resulting in negligible efficiency variation in the entire luminance range.

Original languageEnglish
Pages (from-to)1-8
Number of pages8
JournalElectronic Materials Letters
Volume16
Issue number1
DOIs
StatePublished - 1 Jan 2020

Keywords

  • Blue fluorescent OLEDs
  • Efficiency-lifetime trade off
  • Triplet–triplet fusion

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