Swelling and mechanical properties of glycol chitosan/poly(vinyl alcohol) IPN-type superporous hydrogels

Hyojin Park, Dukjoon Kim

Research output: Contribution to journalArticlepeer-review

58 Scopus citations

Abstract

Glycol chitosan/poly(vinyl alcohol) interpenetrating polymer network type superporous hydrogels were prepared using a gas foaming/freeze-drying method. The effect of the molecular weight of the strengthener, poly(vinyl alcohol) (PVA), on the swelling and mechanical behavior of the superporous hydrogels was investigated. The introduction of a small amount of high molecular weight PVA significantly enhanced the mechanical strength but slightly reduced the swelling capacity. The freezing/thawing (F/T) drying process had a significant effect on the physical properties of the glycol chitosan/PVA superporous hydrogels, because hydrogen bonds were formed between the PVA molecules as a result of the number of F/T cycles. The swelling ratio decreased but the mechanical strength increased with increasing freezing time. However, this effect was not as strong as the number of F/T cycles. The differential scanning calorimetry was used to examine how the thermal behavior associated with the hydrogen bond-induced crystalline structure was affected by the F/T process.

Original languageEnglish
Pages (from-to)662-667
Number of pages6
JournalJournal of Biomedical Materials Research - Part A
Volume78
Issue number4
DOIs
StatePublished - 15 Sep 2006

Keywords

  • Foaming
  • Freezing/thawing process
  • IPN
  • Pore
  • Swelling

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