TY - JOUR
T1 - Recent advances of gallium-based liquid metals
T2 - Properties, patterning strategies, and applications in soft electronics
AU - Shin, Seung Beom
AU - Cho, Jae Hyeok
AU - Lee, Tae Woo
AU - Park, Ji Won
AU - Kim, Myung Gil
N1 - Publisher Copyright:
© 2025 Korean Chemical Society and Wiley-VCH GmbH.
PY - 2025/10
Y1 - 2025/10
N2 - Gallium-based liquid metals (LMs) are emerging as versatile functional materials for next-generation stretchable, wearable, and bio-integrated electronics. Their combined attributes of metallic conductivity, mechanical softness, and room temperature fluidity allow for applications beyond the limitations of conventional rigid conductors. However, despite their promise, intrinsic challenges such as high surface tension, uncontrolled wetting, and poor substrate adhesion remain major obstacles to their practical utilization. Recent advances in LM micro-patterning strategies—including surface energy modulation, chemical treatment, metal adhesion layering, and electrochemical control—have substantially improved printing resolution and device integration. Simultaneously, the development of LM particle composites with tunable rheological and thermal properties has enabled the scalable fabrication of soft electromagnetic interference shielding films and Joule heating devices. LM functionality has been further extended by bio-inspired applications that integrate patterning strategies with neuromorphic electronics, as demonstrated by artificial synaptic interfaces and electrochemically actuated soft robotics. Bridging the intrinsic fluidity of LMs with electronic functionality establishes a pathway toward reconfigurable, adaptive, and human-compatible systems. Despite the remaining challenges, future research directions highlight the potential of gallium-based LMs as a central platform for intelligent, closed-loop soft electronics.
AB - Gallium-based liquid metals (LMs) are emerging as versatile functional materials for next-generation stretchable, wearable, and bio-integrated electronics. Their combined attributes of metallic conductivity, mechanical softness, and room temperature fluidity allow for applications beyond the limitations of conventional rigid conductors. However, despite their promise, intrinsic challenges such as high surface tension, uncontrolled wetting, and poor substrate adhesion remain major obstacles to their practical utilization. Recent advances in LM micro-patterning strategies—including surface energy modulation, chemical treatment, metal adhesion layering, and electrochemical control—have substantially improved printing resolution and device integration. Simultaneously, the development of LM particle composites with tunable rheological and thermal properties has enabled the scalable fabrication of soft electromagnetic interference shielding films and Joule heating devices. LM functionality has been further extended by bio-inspired applications that integrate patterning strategies with neuromorphic electronics, as demonstrated by artificial synaptic interfaces and electrochemically actuated soft robotics. Bridging the intrinsic fluidity of LMs with electronic functionality establishes a pathway toward reconfigurable, adaptive, and human-compatible systems. Despite the remaining challenges, future research directions highlight the potential of gallium-based LMs as a central platform for intelligent, closed-loop soft electronics.
KW - gallium oxide
KW - gallium-based liquid metal
KW - micro-pattern
KW - soft electronics
KW - stretchable electrode
UR - https://www.scopus.com/pages/publications/105017918368
U2 - 10.1002/bkcs.70070
DO - 10.1002/bkcs.70070
M3 - Review article
AN - SCOPUS:105017918368
SN - 0253-2964
VL - 46
SP - 978
EP - 993
JO - Bulletin of the Korean Chemical Society
JF - Bulletin of the Korean Chemical Society
IS - 10
ER -