Abstract
The structural, transport, and magnetic properties of the naturally layered manganese oxide, Sr1.6Sm1.4Mn2O7 (Sm-327), which consists of two [MnO2] bi-layers intertwined with a rock-salt type layer of [(Sr,Sm)2O2] have been investigated. Both a sharp metal-insulator (M-I) transition and an antiferromagnetic transition were found to occur simultaneously at about 118 K. Even in the absence of ferromagnetic ordering the resistance is suppressed remarkably upon applying a magnetic field. These results suggest that the M-I transition and colossal magnetoresistance behavior observed in Sm-327 are not driven mainly by the double exchange mechanism but ascribed rather to the canted antiferromagnetic spin configurations of [MnO2] bi-layers, which eventually leads to the field-induced ferromagnetic ordering.
| Original language | English |
|---|---|
| Pages (from-to) | 61-65 |
| Number of pages | 5 |
| Journal | Solid State Communications |
| Volume | 112 |
| Issue number | 2 |
| DOIs | |
| State | Published - 6 Sep 1999 |