Electrically Tunable Single Polaritonic Quantum Dot at Room Temperature

  • Hyeongwoo Lee
  • , Benjamin G. Whetten
  • , Byong Jae Kim
  • , Ju Young Woo
  • , Yeonjeong Koo
  • , Jinhyuk Bae
  • , Mingu Kang
  • , Taeyoung Moon
  • , Huitae Joo
  • , Sohee Jeong
  • , Jaehoon Lim
  • , Alexander L. Efros
  • , Markus B. Raschke
  • , Matthew Pelton
  • , Kyoung Duck Park

Research output: Contribution to journalArticlepeer-review

6 Scopus citations

Abstract

Exciton-polaritons confined in plasmonic cavities are hybridized light-matter quasiparticles, with distinct optical characteristics compared to plasmons and excitons alone. Here, we demonstrate the electric tunability of a single polaritonic quantum dot operating at room temperature in electric-field tip-enhanced strong coupling spectroscopy. For a single quantum dot in the nanoplasmonic tip cavity with variable dc local electric field, we dynamically control the Rabi frequency with the corresponding polariton emission, crossing weak to strong coupling. We model the observed behaviors based on the quantum confined Stark effect in the strong coupling regime.

Original languageEnglish
Article number133001
JournalPhysical Review Letters
Volume132
Issue number13
DOIs
StatePublished - 29 Mar 2024

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