TY - JOUR
T1 - Convolution Neural Networks for Motion Detection with Electrospun Reversibly-Cross-linkable Polymers and Encapsulated Ag Nanowires
AU - Choi, Su Bin
AU - Shin, Hyun Sik
AU - Kim, Jong Woong
N1 - Publisher Copyright:
© 2023 American Chemical Society
PY - 2023/10/11
Y1 - 2023/10/11
N2 - This paper presents the design, fabrication, and implementation of a novel composite film, a polybutadiene-based urethane (PBU)/AgNW/PBU sensor (PAPS), demonstrating remarkable mechanical stability and precision in motion detection. The sensor capitalizes on the integration of Ag nanowire (AgNW) electrodes into a neutral plane, embedded within a reversibly cross-linkable PBU polymer. The meticulous arrangement confers pore-free and interfaceless sensor formation, resulting in an enhanced mechanical robustness, reproducibility, and long-term reliability. The PBU polymer is subjected to an electrospinning process, followed by sequential Diels-Alder (DA) and retro-DA reactions to produce a planarized encapsulation layer. This pioneering technology, based on electrospinning, allows for more flawless engineering of the neutral plane as compared to conventional film lamination or layer-by-layer spin-coating processes. This encapsulation, matching the thickness of the preformed PBU film, effectively houses the AgNW electrodes. The PAPS outperforms conventional AgNW/PBU sensors (APS) in terms of mechanical stability and bending insensitivity. When affixed to various body parts, the PAPS generates distinctive signal curves, reflecting the specific body part and degree of motion involved. The PAPS sensor’s utility is further magnified by the application of machine learning and deep learning algorithms for signal interpretation. K-means clustering algorithm authenticated the superior reproducibility and consistency of the signals derived from the PAPS over the APS. Deep learning algorithms, including a singular 1D convolutional neural network (1D CNN), long short-term memory (LSTM) network, and dual-layered combinations of 1D CNN + LSTM and LSTM + 1D CNN, were deployed for signal classification. The singular 1D CNN model displayed a classification accuracy exceeding 98%. The PAPS sensor signifies a pivotal development in the field of intelligent motion sensors.
AB - This paper presents the design, fabrication, and implementation of a novel composite film, a polybutadiene-based urethane (PBU)/AgNW/PBU sensor (PAPS), demonstrating remarkable mechanical stability and precision in motion detection. The sensor capitalizes on the integration of Ag nanowire (AgNW) electrodes into a neutral plane, embedded within a reversibly cross-linkable PBU polymer. The meticulous arrangement confers pore-free and interfaceless sensor formation, resulting in an enhanced mechanical robustness, reproducibility, and long-term reliability. The PBU polymer is subjected to an electrospinning process, followed by sequential Diels-Alder (DA) and retro-DA reactions to produce a planarized encapsulation layer. This pioneering technology, based on electrospinning, allows for more flawless engineering of the neutral plane as compared to conventional film lamination or layer-by-layer spin-coating processes. This encapsulation, matching the thickness of the preformed PBU film, effectively houses the AgNW electrodes. The PAPS outperforms conventional AgNW/PBU sensors (APS) in terms of mechanical stability and bending insensitivity. When affixed to various body parts, the PAPS generates distinctive signal curves, reflecting the specific body part and degree of motion involved. The PAPS sensor’s utility is further magnified by the application of machine learning and deep learning algorithms for signal interpretation. K-means clustering algorithm authenticated the superior reproducibility and consistency of the signals derived from the PAPS over the APS. Deep learning algorithms, including a singular 1D convolutional neural network (1D CNN), long short-term memory (LSTM) network, and dual-layered combinations of 1D CNN + LSTM and LSTM + 1D CNN, were deployed for signal classification. The singular 1D CNN model displayed a classification accuracy exceeding 98%. The PAPS sensor signifies a pivotal development in the field of intelligent motion sensors.
KW - Ag nanowire
KW - cognitive convolutional neural networks
KW - Diels−Alder
KW - electrospinning
KW - polybutadiene-based urethane
UR - https://www.scopus.com/pages/publications/85175587257
U2 - 10.1021/acsami.3c11918
DO - 10.1021/acsami.3c11918
M3 - Article
C2 - 37782487
AN - SCOPUS:85175587257
SN - 1944-8244
VL - 15
SP - 47591
EP - 47603
JO - ACS Applied Materials and Interfaces
JF - ACS Applied Materials and Interfaces
IS - 40
ER -